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Temperature and conversion patterns in a network of catalytic reactors for methanol synthesis with different switch strategies (Articolo in rivista)
- Type
- Label
- Temperature and conversion patterns in a network of catalytic reactors for methanol synthesis with different switch strategies (Articolo in rivista) (literal)
- Anno
- 2010-01-01T00:00:00+01:00 (literal)
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#doi
- 10.1016/j.ces.2010.04.043 (literal)
- Alternative label
Mancusi, E; Altimari, P; Crescitelli, S; Russo L. (2010)
Temperature and conversion patterns in a network of catalytic reactors for methanol synthesis with different switch strategies
in Chemical engineering science
(literal)
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#autori
- Mancusi, E; Altimari, P; Crescitelli, S; Russo L. (literal)
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- Rivista
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#numeroFascicolo
- Note
- ISI Web of Science (WOS) (literal)
- Scopus (literal)
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#affiliazioni
- Erasmo Mancusi a, PietroAltimari b, SilvestroCrescitelli c, LuciaRusso d,
a Facolt?a diIngegneria,Universit?a delSannio,PiazzaRoma,82100Benevento,Italy
b Dipartimento diIngegneriaChimicaAlimentareUniversit?a diSalerno,ViaPonteDonMelillo,84084Fisciano(SA),Italy
c Dipartimento d'IngegneriaChimicaUniversit?a ''FedericoII''PiazzaleTecchio80,I-80125Napoli,Italy
d CNR, IstitutodelleRicerchesullaCombustione,P.leTecchio80,Napoli80125,Italy (literal)
- Titolo
- Temperature and conversion patterns in a network of catalytic reactors for methanol synthesis with different switch strategies (literal)
- Abstract
- A network of connected catalyticreactorswithperiodicallyswitchedinletandoutletsectionsis
numericallystudiedforreversibleexothermicreactions.Themethanolsynthesisisselectedas
representativeprocessexampleandtwodifferentswitchstrategiesarecomparedwiththeobjectiveof
overcomingtheconversionlimitsimposedbythermodynamicequilibrium.Thefirststrategy,whichis
the mostconsideredinliterature,consistsofperiodicallyswitchingthefeedtothesecondreactorofthe
currentreactorsequencewhilethesecondstrategyisimplementedbyperiodicallyswitchingthefeed
to thelastreactorofthecurrentsequence.Periodicregimescorrespondingtosinglesquare-like
temperaturewavestravellingoverthecatalyticbedandcharacterizedbycomparablemethanol
conversionvaluesaredetectedforboththeconsideredstrategies.Theseregimesexhibit,however,a
significantlylargerdomainofexistenceforthesecondstrategy.Moreover,thesecondstrategygivesrise
to otherperiodicregimescorrespondingtospatiotemporaltemperaturepatternscharacterizedby
differentspatialandtemporalperiodicity.Thesepatternsariseintheformoftemperaturewavetrains
and ensuremethanolconversionvaluessignificantlylargerthanthosefoundunderperiodicregimes
characterizedbysingletemperaturewaves. (literal)
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