Combining M- and L-edge resonant inelastic x-ray scattering for studies of 3d transition metal compounds (Articolo in rivista)

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Label
  • Combining M- and L-edge resonant inelastic x-ray scattering for studies of 3d transition metal compounds (Articolo in rivista) (literal)
Anno
  • 2008-01-01T00:00:00+01:00 (literal)
Alternative label
  • Chiuzbaian, SG; Schmitt, T; Matsubara, M; Kotani, A; Ghiringhelli, G; Dallera, C; Tagliaferri, A; Braicovich, L; Scagnoli, V; Brookes, NB; Staub, U; Patthey, L (2008)
    Combining M- and L-edge resonant inelastic x-ray scattering for studies of 3d transition metal compounds
    (literal)
Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#autori
  • Chiuzbaian, SG; Schmitt, T; Matsubara, M; Kotani, A; Ghiringhelli, G; Dallera, C; Tagliaferri, A; Braicovich, L; Scagnoli, V; Brookes, NB; Staub, U; Patthey, L (literal)
Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#numeroVolume
  • 78 (literal)
Note
  • ISI Web of Science (WOS) (literal)
Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#affiliazioni
  • \"[Chiuzbaian, S. G.] Univ Paris 06, UPMC, Lab Chim Phys Mat & Rayonnement, CNRS UMR 7614, F-75005 Paris, France; [Schmitt, T.; Staub, U.; Patthey, L.] Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland; [Matsubara, M.] Univ Montpellier 2, Verres & Nanomat UMR 5587, Lab Colloides, F-34095 Montpellier, France; [Kotani, A.] RIKEN Spring8, Sayo, Hyogo 6795148, Japan; [Kotani, A.] High Energy Accelerator Res Org, IMSS, Photon Factory, Tsukuba, Ibaragi 3050801, Japan; [Ghiringhelli, G.] Politecn Milan, Dipartimento Fis, CNR INFM Coherentia, I-20133 Milan, Italy; [Dallera, C.] Politecn Milan, Dipartimento Fis, CNR INFM ULTRAS, I-20133 Milan, Italy; [Tagliaferri, A.; Braicovich, L.] Politecn Milan, Dipartimento Fis, CNR INFM SOFT, I-20133 Milan, Italy; [Ghiringhelli, G.] Politecn Milan, Dipartimento Fis, SOFT, I-20133 Milan, Italy; [Scagnoli, V.; Brookes, N. B.] European Synchrotron Radiat Facil, F-38043 Grenoble, France (literal)
Titolo
  • Combining M- and L-edge resonant inelastic x-ray scattering for studies of 3d transition metal compounds (literal)
Abstract
  • Resonant inelastic x-ray scattering (RIXS) measurements performed jointly across the M-2,M-3 and L-3 absorption thresholds are used to study CoO local electronic structure and are supported by model calculations. The high-resolution experimental data provide a precise set of parameters to describe the correlated response of valence electrons. The same core-hole independent set of parameters within the single impurity Anderson model is used to describe both the M (3p-3d) and L (2p-3d) resonances. This work shows that combining M and L scattering data provides an enhanced contrast view of the spectral weights. Measured M-2,M-3-RIXS spectra are observed to be free of charge-transfer or normal fluorescence contributions. Moreover the cross section of M-RIXS final states with change in spin multiplicity is low. Combining this information with L-edge studies establishes an appealing means of making a better separation between on-site and intersite (ligand to metal) electronic excitations. Experimental and theoretical features specific to RIXS studies performed at M and L edges are summarized as a basis for future studies on complex transition metal compounds. (literal)
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