http://www.cnr.it/ontology/cnr/individuo/prodotto/ID291788
Collective Autoionization in Multiply-Excited Systems: A novel ionization process observed in Helium Nanodroplets (Articolo in rivista)
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- Label
- Collective Autoionization in Multiply-Excited Systems: A novel ionization process observed in Helium Nanodroplets (Articolo in rivista) (literal)
- Anno
- 2014-01-01T00:00:00+01:00 (literal)
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#doi
- 10.1038/srep03621 (literal)
- Alternative label
LaForge, A. C.; Drabbels, M.; Brauer, N. B.; Coreno, M.; Devetta, M.; Di Fraia, M.; Finetti, P.; Grazioli, C.; Katzy, R.; Lyamayev, V.; Mazza, T.; Mudrich, M.; O'Keeffe, P.; Ovcharenko, Y.; Piseri, P.; Plekan, O.; Prince, K. C.; Richter, R.; Stranges, S.; Callegari, C.; Moeller, T.; Stienkemeier, F. (2014)
Collective Autoionization in Multiply-Excited Systems: A novel ionization process observed in Helium Nanodroplets
in Scientific reports (Nature Publishing Group)
(literal)
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#autori
- LaForge, A. C.; Drabbels, M.; Brauer, N. B.; Coreno, M.; Devetta, M.; Di Fraia, M.; Finetti, P.; Grazioli, C.; Katzy, R.; Lyamayev, V.; Mazza, T.; Mudrich, M.; O'Keeffe, P.; Ovcharenko, Y.; Piseri, P.; Plekan, O.; Prince, K. C.; Richter, R.; Stranges, S.; Callegari, C.; Moeller, T.; Stienkemeier, F. (literal)
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- ISI Web of Science (WOS) (literal)
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#affiliazioni
- University of Freiburg; Ecole Polytechnique Federale de Lausanne; CNR IMIP Rome; University of Milan; University of Trieste; Elettra Sincrotrone Trieste; Sapienza University Rome (literal)
- Titolo
- Collective Autoionization in Multiply-Excited Systems: A novel ionization process observed in Helium Nanodroplets (literal)
- Abstract
- Free electron lasers (FELs) offer the unprecedented capability to study reaction dynamics and image the structure of complex systems. When multiple photons are absorbed in complex systems, a plasma-like state is formed where many atoms are ionized on a femtosecond timescale. If multiphoton absorption is resonantly-enhanced, the system becomes electronically-excited prior to plasma formation, with subsequent decay paths which have been scarcely investigated to date. Here, we show using helium nanodroplets as an example that these systems can decay by a new type of process, named collective autoionization. In addition, we show that this process is surprisingly efficient, leading to ion abundances much greater than that of direct single-photon ionization. This novel collective ionization process is expected to be important in many other complex systems, e.g. macromolecules and nanoparticles, exposed to high intensity radiation fields. (literal)
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