Observation of Distinct Bulk and Surface Chemical Environments in a Topological Insulator under Magnetic Doping (Articolo in rivista)

Type
Label
  • Observation of Distinct Bulk and Surface Chemical Environments in a Topological Insulator under Magnetic Doping (Articolo in rivista) (literal)
Anno
  • 2014-01-01T00:00:00+01:00 (literal)
Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#doi
  • 10.1021/jp502729u (literal)
Alternative label
  • Vobornik, Ivana and Panaccione, Giancarlo and Fujii, Jun and Zhu, Zhi-Huai and Offi, Francesco and Salles, Benjamin R. and Borgatti, Francesco and Torelli, Piero and Rueff, Jean Pascal and Ceolin, Denis and Artioli, Alberto and Unnikrishnan, Manju and Levy, Giorgio and Marangolo, Massimiliano and Eddrief, Mamhoud and Krizmancic, Damjan and Ji, Huiwen and Damascelli, Andrea and van der Laan, Gerrit and Egdell, Russell G. and Cava, Robert J. (2014)
    Observation of Distinct Bulk and Surface Chemical Environments in a Topological Insulator under Magnetic Doping
    in Journal of physical chemistry. C
    (literal)
Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#autori
  • Vobornik, Ivana and Panaccione, Giancarlo and Fujii, Jun and Zhu, Zhi-Huai and Offi, Francesco and Salles, Benjamin R. and Borgatti, Francesco and Torelli, Piero and Rueff, Jean Pascal and Ceolin, Denis and Artioli, Alberto and Unnikrishnan, Manju and Levy, Giorgio and Marangolo, Massimiliano and Eddrief, Mamhoud and Krizmancic, Damjan and Ji, Huiwen and Damascelli, Andrea and van der Laan, Gerrit and Egdell, Russell G. and Cava, Robert J. (literal)
Pagina inizio
  • 12333 (literal)
Pagina fine
  • 12339 (literal)
Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#numeroVolume
  • 118 (literal)
Rivista
Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#numeroFascicolo
  • 23 (literal)
Note
  • ISI Web of Science (WOS) (literal)
Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#affiliazioni
  • Vobornik, I (Reprint Author), CNR, IOM, Lab TASC, Area Sci Pk,S-S-14,Km 163-5, I-34149 Trieste, Italy. Vobornik, Ivana; Panaccione, Giancarlo; Fujii, Jun; Salles, Benjamin R.; Torelli, Piero; Artioli, Alberto; Krizmancic, Damjan, CNR, IOM, Lab TASC, I-34149 Trieste, Italy. Zhu, Zhi-Huai; Levy, Giorgio; Damascelli, Andrea, Univ British Columbia, Dept Phys & Astron, Vancouver, BC V6T 1Z1, Canada. Offi, Francesco; van der Laan, Gerrit, Univ Roma Tre, Dipartimento Sci, I-00146 Rome, Italy. Borgatti, Francesco, CNR, ISMN, I-40129 Bologna, Italy. Rueff, Jean Pascal; Ceolin, Denis, Synchrotron SOLEIL, F-91192 Gif Sur Yvette, France. Rueff, Jean Pascal, Univ Paris 06, CNRS, Lab Chim Phys Mat & Rayonnement, F-75005 Paris, France. Marangolo, Massimiliano; Eddrief, Mamhoud, UPMC, CNRS, Inst NanoSci Paris, UMR 7588, F-75252 Paris 5, France. Ji, Huiwen; Cava, Robert J., Princeton Univ, Dept Chem, Princeton, NJ 08544 USA. Levy, Giorgio; Damascelli, Andrea, Univ British Columbia, Quantum Matter Inst, Vancouver, BC V6T 1Z4, Canada. Diamond Light Source, Didcot OX11 0DE, Oxon, England. Egdell, Russell G., Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England. Unnikrishnan, Manju, Abdus Salaam Int Ctr Theoret Phys, I-34100 Trieste, Italy. (literal)
Titolo
  • Observation of Distinct Bulk and Surface Chemical Environments in a Topological Insulator under Magnetic Doping (literal)
Abstract
  • The influence of magnetic dopants on the electronic and chemical environments in topological insulators (TIs) is a key factor when considering possible spintronic applications based on topological surface state properties. Here we provide spectroscopic evidence for the presence of distinct chemical and electronic behavior for surface and bulk magnetic doping of Bi2Te3. The inclusion of Mn in the bulk of Bi2Te3 induces a genuine dilute ferromagnetic state, with reduction of the bulk band gap as the Mn content is increased. Deposition of Fe on the Bi2Te3 surface, on the other hand, favors the formation of iron telluride already at coverages as low as 0.07 monolayer, as a consequence of the reactivity of the Te-rich surface. Our results identify the factors that need to be controlled in the realization of magnetic nanosystems and interfaces based on TIs. (literal)
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