http://www.cnr.it/ontology/cnr/individuo/prodotto/ID273263
Excitation Spectra of Transition-Metal Atoms on the Ag (100) Surface Controlled by Hund's Exchange (Articolo in rivista)
- Type
- Label
- Excitation Spectra of Transition-Metal Atoms on the Ag (100) Surface Controlled by Hund's Exchange (Articolo in rivista) (literal)
- Anno
- 2013-01-01T00:00:00+01:00 (literal)
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#doi
- 10.1103/PhysRevLett.110.186404 (literal)
- Alternative label
S. Gardonio, M. Karolak, T. O. Wehling, L. Petaccia, S. Lizzit, A. Goldoni, A. I. Lichtenstein, and C. Carbone (2013)
Excitation Spectra of Transition-Metal Atoms on the Ag (100) Surface Controlled by Hund's Exchange
in Physical review letters (Print)
(literal)
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#autori
- S. Gardonio, M. Karolak, T. O. Wehling, L. Petaccia, S. Lizzit, A. Goldoni, A. I. Lichtenstein, and C. Carbone (literal)
- Pagina inizio
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#numeroVolume
- Rivista
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- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#affiliazioni
- Materials Research Laboratory, University of Nova Gorica, Vipavska 13, 5000 Nova Gorica, Slovenia
I. Institut für Theoretische Physik, Universität Hamburg, Jungiusstraße 9, D-20355 Hamburg, Germany
Institut für Theoretische Physik, Universität Bremen, Otto-Hahn-Allee 1, D-28359 Bremen, Germany
Bremen Center for Computational Materials Science, Universität Bremen, Am Fallturm 1a, 28359 Bremen, Germany
Elettra Sincrotrone Trieste, Strada Statale 14 km 163.5, 34149 Trieste, Italy
Istituto di Struttura della Materia, Consiglio Nazionale delle Ricerche, Basovizza, I-34149 Trieste, Italy (literal)
- Titolo
- Excitation Spectra of Transition-Metal Atoms on the Ag (100) Surface Controlled by Hund's Exchange (literal)
- Abstract
- We report photoemission experiments revealing the valence electron spectral function of Mn, Fe, Co, and Ni atoms on the Ag (100) surface. The series of spectra shows splittings of higher energy features which decrease with the filling of the 3d shell and a highly nonmonotonic evolution of spectral weight near the Fermi edge. First principles calculations demonstrate that two manifestations of Hund's exchange J are responsible for this evolution. First, there is a monotonic reduction of the effective exchange splittings with increasing filling of the 3d shell. Second, the amount of charge fluctuations and, thus, the weight of quasiparticle peaks at the Fermi level varies nonmonotonically through this 3d series due to a distinct occupancy dependence of effective charging energies Ueff. (literal)
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