http://www.cnr.it/ontology/cnr/individuo/prodotto/ID24604
X-ray absorption and diffraction studies of Pr3+, Tb3+ and Er3+-activated silica gels. (Articolo in rivista)
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- X-ray absorption and diffraction studies of Pr3+, Tb3+ and Er3+-activated silica gels. (Articolo in rivista) (literal)
- Anno
- 2003-01-01T00:00:00+01:00 (literal)
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- Rocca F.; Armellini C.; Ferrari M.; Dalba G.; Diab N.; Kuzmin A.; Monti F. (literal)
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- ISI Web of Science (WOS) (literal)
- Titolo
- X-ray absorption and diffraction studies of Pr3+, Tb3+ and Er3+-activated silica gels. (literal)
- Abstract
- Rare-earth (Pr3+, Tb3+, Er3+) doped silica xerogels were studied by x-ray absorption spectroscopy and x-ray diffraction. A change of the local environment around rare-earth ions upon xerogel densification at 900-950 degreesC and co-doping with aluminum ions was determined from the
rare-earths L-3-edge EXAFS signals. The densification process induces a decrease of the coordination number and a compression and deformation of the first coordination shell, composed of oxygen atoms. The second coordination shell, composed of silicon and/or aluminum ions, also
experiences some modification, which is attributed mainly to a shortening of the shell radius. No evidence of clustering of rare-earth ions upon densification was observed. X-ray diffraction data on Tb-doped gels confirm the EXAFS results
(literal)
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