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Real-time observation of ultrafast Rabi oscillations between excitons and plasmons in metal nanostructures with J-aggregates (Articolo in rivista)
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- Real-time observation of ultrafast Rabi oscillations between excitons and plasmons in metal nanostructures with J-aggregates (Articolo in rivista) (literal)
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- 2013-01-01T00:00:00+01:00 (literal)
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#doi
- 10.1038/NPHOTON.2012.340 (literal)
- Alternative label
Vasa, P.(ab) , Wang, W.(a), Pomraenke, R.(a), Lammers, M.(a), Maiuri, M.(c), Manzoni, C.(c), Cerullo, G.(c), Lienau, C.(a) (2013)
Real-time observation of ultrafast Rabi oscillations between excitons and plasmons in metal nanostructures with J-aggregates
in Nature photonics (Print)
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- Vasa, P.(ab) , Wang, W.(a), Pomraenke, R.(a), Lammers, M.(a), Maiuri, M.(c), Manzoni, C.(c), Cerullo, G.(c), Lienau, C.(a) (literal)
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- http://www.nature.com/nphoton/journal/v7/n2/full/nphoton.2012.340.html (literal)
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- a Institut für Physik, Center of Interface Science, Carl von Ossietzky Universität, 26129 Oldenburg, Germany
b Department of Physics, Indian Institute of Technology Bombay, 400076 Mumbai, India
c IFN-CNR, Dipartimento di Fisica, Politecnico di Milano, 20133 Milan, Italy (literal)
- Titolo
- Real-time observation of ultrafast Rabi oscillations between excitons and plasmons in metal nanostructures with J-aggregates (literal)
- Abstract
- Surface plasmon polaritons (SPPs), optical excitations at the interface between a metal and a dielectric, carry significant potential for guiding and manipulating light on the nanoscale(1-3). However, their weak optical nonlinearities hinder active device fabrication, for example, for all-optical switching(4-7) or information processing(8,9). Recently, strong optical dipole coupling has been demonstrated between SPPs and nonlinear quantum emitters with normal mode splittings of up to 700 meV (refs 10-15). The predicted ultrafast energy transfer between quantum emitters and SPP fields could be a crucial microscopic mechanism for switching light by light on the nanoscale. Here, we present the first real-time observation of ultrafast Rabi oscillations in a J-aggregate/metal nanostructure, indicating coherent energy transfer between excitonic quantum emitters and SPP fields. We demonstrate coherent manipulation of the coupling energy by controlling the exciton density on a 10 fs timescale, which represents a step towards coherent, all-optical ultrafast plasmonic circuits and devices. (literal)
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