http://www.cnr.it/ontology/cnr/individuo/prodotto/ID228892
AB-INITIO RO-VIBRATIONAL LEVELS OF H-3(+) BEYOND THE BORN-OPPENHEIMER APPROXIMATION (Articolo in rivista)
- Type
- Label
- AB-INITIO RO-VIBRATIONAL LEVELS OF H-3(+) BEYOND THE BORN-OPPENHEIMER APPROXIMATION (Articolo in rivista) (literal)
- Anno
- 1995-01-01T00:00:00+01:00 (literal)
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#doi
- 10.1016/0009-2614(94)01301-B (literal)
- Alternative label
DINELLI, BM (DINELLI, BM); LESUEUR, CR (LESUEUR, CR); TENNYSON, J (TENNYSON, J); AMOS, RD (AMOS, RD) (1995)
AB-INITIO RO-VIBRATIONAL LEVELS OF H-3(+) BEYOND THE BORN-OPPENHEIMER APPROXIMATION
in Chemical physics letters (Print)
(literal)
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#autori
- DINELLI, BM (DINELLI, BM); LESUEUR, CR (LESUEUR, CR); TENNYSON, J (TENNYSON, J); AMOS, RD (AMOS, RD) (literal)
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- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#numeroVolume
- Rivista
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#numeroFascicolo
- Note
- ISI Web of Science (WOS) (literal)
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#affiliazioni
- UNIV LONDON UNIV COLL,DEPT PHYS & ASTRON,GOWER ST,LONDON WC1E 6BT,ENGLAND.
UNIV CAMBRIDGE,CHEM LABS,CAMBRIDGE CB2 1EW,ENGLAND (literal)
- Titolo
- AB-INITIO RO-VIBRATIONAL LEVELS OF H-3(+) BEYOND THE BORN-OPPENHEIMER APPROXIMATION (literal)
- Abstract
- The value of the adiabatic correction to the Born-Oppenheimer electronic energy is calculated as a function of geometry for H3+ using SCF wavefunctions. A mass-dependent adiabatic function is combined with the near-Born-Oppenheimer electronic structure calculations of Rohse, Kutzelnigg, Jaquet and Klopper and the rotation-vibration energy levels of H3+ and D3+ are calculated. The levels for H3+ are significantly better than any previous ab initio estimates but are less accurate than those obtained by recent spectroscopically determined effective H3+ potentials. The adiabatic correction is less important for the heavier D3+. For both ions rotational levels are obtained to near experimental accuracy. Small, systematic shifts in the vibrational bands may be attributable to residual errors in the Born-Oppenheimer potential. (literal)
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