http://www.cnr.it/ontology/cnr/individuo/prodotto/ID20036
Snow-to-air exchanges of mercury in an Arctic seasonal snow pack in Ny-Alesund, Svalbard. (Articolo in rivista)
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- Snow-to-air exchanges of mercury in an Arctic seasonal snow pack in Ny-Alesund, Svalbard. (Articolo in rivista) (literal)
- Anno
- 2005-01-01T00:00:00+01:00 (literal)
- Alternative label
Ferrari PC., Gauchard PA., Aspmo K., Dommergue A., Magand O., Bahlmann E., Nagorski S., Temme C., Ebinghaus R., Steffen A., Banic C., Berg T., Planchon F., Barbante C., Cescon P., Boutron CF. (2005)
Snow-to-air exchanges of mercury in an Arctic seasonal snow pack in Ny-Alesund, Svalbard.
in Atmospheric environment (1994)
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- Ferrari PC., Gauchard PA., Aspmo K., Dommergue A., Magand O., Bahlmann E., Nagorski S., Temme C., Ebinghaus R., Steffen A., Banic C., Berg T., Planchon F., Barbante C., Cescon P., Boutron CF. (literal)
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peak in Gaseous Elemental Mercury (GEM) emission flux from the snow to the atmosphere has been measured just few
hours after an Atmospheric Mercury Depletion Event (AMDE) recorded on 22 April 2004. Surprisingly, this peak in
GEM emitted after this AMDE did not correspond to any increase in Hg concentration in snow surface. A peak in
GEM flux after an AMDE was observed only for this single event but not for the four other AMDEs recorded during
this spring period.
In the snow pack which is seasonal and about 40 cm depth above permafrost, Hg is involved in both production and
incorporation processes. The incorporation was evaluated to ~540 pgm2 h. (literal)
- Note
- ISI Web of Science (WOS) (literal)
- Titolo
- Snow-to-air exchanges of mercury in an Arctic seasonal snow pack in Ny-Alesund, Svalbard. (literal)
- Abstract
- The study of mercury (Hg) cycle in Arctic regions is a major subject of concern due to the dramatic increases of Hg
concentrations in ecosystem in the last few decades. The causes of such increases are still in debate, and an important
way to improve our knowledge on the subject is to study the exchanges of Hg between atmosphere and snow during
springtime. We organized an international study from 10 April to 10 May 2003 in Ny-AÚ lesund, Svalbard, in order to
assess these fluxes through measurements and derived calculations.
Snow-to-air emission fluxes of Hg were measured using the flux chamber technique between ~0 and 50 ngm-2 h-1. A
peak in Gaseous Elemental Mercury (GEM) emission flux from the snow to the atmosphere has been measured just few
hours after an Atmospheric Mercury Depletion Event (AMDE) recorded on 22 April 2004. Surprisingly, this peak in
GEM emitted after this AMDE did not correspond to any increase in Hg concentration in snow surface. A peak in
GEM flux after an AMDE was observed only for this single event but not for the four other AMDEs recorded during
this spring period.
In the snow pack which is seasonal and about 40 cm depth above permafrost, Hg is involved in both production and
incorporation processes. The incorporation was evaluated to ~540 pgm2 h. Outside of AMDE periods, Hg flux from
the snow surface to the atmosphere was the consequence of GEM production in the air of snow and was about
~1550 ngm-2 h-1, with a contribution of deeper snow layers evaluated to ~0.36.5 ngm-2 h-1. The major part of GEM production is then mainly a surface phenomenon. The internal production of GEM was largely increasing when
snow temperatures were close to melting, indicating a chemical process occurring in the quasi-liquid layer at the surface
of snow grains. (literal)
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