http://www.cnr.it/ontology/cnr/individuo/prodotto/ID17750
Chemoenzymatic Synthesis of Fluorescent and Colored Polyesters (Articolo in rivista)
- Type
- Label
- Chemoenzymatic Synthesis of Fluorescent and Colored Polyesters (Articolo in rivista) (literal)
- Anno
- 2011-01-01T00:00:00+01:00 (literal)
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#doi
- 10.1002/cctc.201000327 (literal)
- Alternative label
Navarra, Cristina; Marzorati, Mattia; Danieli, Bruno; Riva, Sergio (2011)
Chemoenzymatic Synthesis of Fluorescent and Colored Polyesters
in ChemCatChem (Print)
(literal)
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#autori
- Navarra, Cristina; Marzorati, Mattia; Danieli, Bruno; Riva, Sergio (literal)
- Pagina inizio
- Pagina fine
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#numeroVolume
- Rivista
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#pagineTotali
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#numeroFascicolo
- Note
- ISI Web of Science (WoS) (literal)
- ISI Web of Science (WOS) (literal)
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#affiliazioni
- Ist Chim Riconoscimento Mol; University of Milan (literal)
- Titolo
- Chemoenzymatic Synthesis of Fluorescent and Colored Polyesters (literal)
- Abstract
- A simple chemoenzymatic strategy for the synthesis of colored and fluorescent poly(epsilon-caprolactone) esters has been developed. The procedure involves first the reaction of a functionalized primary amine with epsilon-caprolactone, to give an amide with a terminal primary hydroxy group, followed by an enzymatic ring-opening polymerization catalyzed by Novozym 435. The proposed method is easy to handle and is suitable for the incorporation of different amines, as it shown for the yellow compound N-deacetylthiocolchicine and the fluorescent amines 4-(2-aminoethylamino)-7-(N,N-dimethylsulfamoyl) benzofurazan and dansylcadaverine. A similar strategy is considered for the synthesis of poly(epsilon-caprolactone) esters, employing alcohols as initiators of the reaction. In this case, an intermediate ester carrying a terminal primary hydroxy group cannot be isolated and the reaction forms directly the desired polymers. (literal)
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