Optical investigation of LaMnO(3) thin films: a study of the 2-eV band (Articolo in rivista)

Type
Label
  • Optical investigation of LaMnO(3) thin films: a study of the 2-eV band (Articolo in rivista) (literal)
Anno
  • 2011-01-01T00:00:00+01:00 (literal)
Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#doi
  • 10.1140/epjb/e2011-10945-0 (literal)
Alternative label
  • Nucara, A ; Granozio, FM; Radovic, M; Vitucci, FM; Maselli, P; Fittipaldi, R; Vecchione, A; Calvani, P (2011)
    Optical investigation of LaMnO(3) thin films: a study of the 2-eV band
    in The European physical journal. B, Condensed matter physics (Print)
    (literal)
Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#autori
  • Nucara, A ; Granozio, FM; Radovic, M; Vitucci, FM; Maselli, P; Fittipaldi, R; Vecchione, A; Calvani, P (literal)
Pagina inizio
  • 435 (literal)
Pagina fine
  • 441 (literal)
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  • 79 (literal)
Rivista
Note
  • ISI Web of Science (WOS) (literal)
Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#affiliazioni
  • CNR-SPIN and Dipartimento di Fisica, Universit`a di Roma La Sapienza, Piazzale A. Moro 2, 00185 Roma, Italy CNR-SPIN and Dipartimento di Scienze Fisiche, Universit´a degli Studi Federico II Complesso Universitario di Monte Sant'Angelo via Cinthia 80126, Napoli, Italy CNR-SPIN and Dipartimento di Fisica E.R. Caianiello, Universit`a di Salerno, via Ponte don Melillo, 84084 Fisciano, Italy (literal)
Titolo
  • Optical investigation of LaMnO(3) thin films: a study of the 2-eV band (literal)
Abstract
  • We measure the transmittance of LaMnO3 (LMO) thin films in the spectral range from 10 000 to 38 000 cm-1 as a function of temperature. The optical conductivity obtained from the transmittance data is decomposed into five Drude-Lorentz contributions: three of them show evident changes below the N´eel temperature TN ? 140 K. We discuss the band assignment in the framework of the tight-binding and of the orbitally degenerate Hubbard models. Our results ascribe the overall low-frequency spectrum of LMO to charge-transfer mechanisms involving the t2g and eg electrons of the Mn ions, without invoking the presence of excitonic contributions. This finding definitely promotes a Mott-Hubbard scenario for LMO and provides an estimate of the Hamiltonian parameters. (literal)
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