http://www.cnr.it/ontology/cnr/individuo/prodotto/ID52048
Experimental evidence of a two step reversible absorption/desorption process in ruthenium phthalocyanine gas sensing films by in situ energy dispersive x-ray reflectometry (Articolo in rivista)
- Type
- Label
- Experimental evidence of a two step reversible absorption/desorption process in ruthenium phthalocyanine gas sensing films by in situ energy dispersive x-ray reflectometry (Articolo in rivista) (literal)
- Anno
- 2005-01-01T00:00:00+01:00 (literal)
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#doi
- 10.1063/1.1874311 (literal)
- Alternative label
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#autori
- Generosi A. (1); Paci B. (1); Rossi Albertini V. (1); Perfetti P. (1); Pennesi G. (2); Paoletti A.M. (2); Rossi G. (2); Capobianchi A. (2); Caminiti R. (3) (literal)
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- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#numeroVolume
- Rivista
- Note
- ISI Web of Science (WOS) (literal)
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#affiliazioni
- (1) Istituto di Struttura della Materia-Area di Ricerca di Tor Vergata, Roma, Italy;
(2) Istituto di Struttura della Materia-Area di Ricerca di Montelibretti, Monterotondo Stazione, Roma, Italy;
(3) Dipartimento di Chimica, Università \"La Sapienza\" di Roma e sezione INFM, Roma, Italy (literal)
- Titolo
- Experimental evidence of a two step reversible absorption/desorption process in ruthenium phthalocyanine gas sensing films by in situ energy dispersive x-ray reflectometry (literal)
- Abstract
- An in situ energy dispersive x-ray reflectivity technique was used to study the morphological changes of gas sensing thin films of ruthenium phtalocyanine (RuPc)2 induced by gas absorption/desorption processes. The time-resolved collection of reflectivity spectra during the exposure of each film to a gas flux of nitrogen oxides provided the evolution of the morphological parameters (thickness and roughness). The gas absorption process develops in two stages: The first induces morphological changes characteristic of a surface (adsorption) process, while the second is dominated by a bulk effect. This two-step behavior is also observed in the desorption process: When the thermal treatment is performed at 130 °C, the gas is released from the bulk only. Conversely, at higher temperatures, the gas is fully released, i.e., also from the surface, and the initial film thickness is regained. Finally, a further in situ study upon a second absorption treatment was carried out: In this case, only the film bulk diffusion process takes place. (literal)
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