http://www.cnr.it/ontology/cnr/individuo/prodotto/ID42629
Development of a dual functional structured catalyst for partial oxidation of methane to syngas (Articolo in rivista)
- Type
- Label
- Development of a dual functional structured catalyst for partial oxidation of methane to syngas (Articolo in rivista) (literal)
- Anno
- 2005-01-01T00:00:00+01:00 (literal)
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#doi
- 10.1016/j.cattod.2005.06.058 (literal)
- Alternative label
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#autori
- Cimino S., Landi G., Lisi L. and Russo G (literal)
- Pagina inizio
- Pagina fine
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#numeroVolume
- Rivista
- Note
- Scopu (literal)
- ISI Web of Science (WOS) (literal)
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#affiliazioni
- CNR ISTITUTO DI RICERCHE SULLA COMBUSTIONE
UNIVERSITA' DEGLI STUDI DI NAPOLI FEDERICO II DIP. INGEGNERIA CHIMICA (literal)
- Titolo
- Development of a dual functional structured catalyst for partial oxidation of methane to syngas (literal)
- Abstract
- Rh-LaCoO3 structured catalysts for the oxidative production of syngas from methane were developed by deposition of the active components on La-g-Al2O3 washcoated honeycomb monoliths. SEM/EDS analysis showed a good adhesion of the washcoat layer and a uniform distribution of La and Co, while Rh was favourably located on the outer shell. Catalytic partial oxidation of methane was tested under both isothermal and pseudo-adiabatic conditions showing that the process can be conducted with high yield and selectivity and stable performance at short contact times over the novel catalysts, characterised by a limited content of noble metal and no need for pre-reduction. Further experiments of CO2 autothermal reforming indicated the possibility to enhance CO production and to reduce the H2 /CO ratio through secondary endothermic reactions consuming CO2, which are autothermally self-sustained in a single catalytic reactor operated at short contact time by the heat generated through partial oxidation reactions. (literal)
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- Autore CNR
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