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Metal-organic coordination interactions in Fe-Terephthalic acid networks on Cu(100) (Articolo in rivista)

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Metal-organic coordination interactions in Fe-Terephthalic acid networks on Cu(100) (Articolo in rivista) (literal)

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Alternative label

Tait, SL; Wang, Y; Costantini, G; Lin, N; Baraldi, A; Esch, F; Petaccia, L; Lizzit, S; Kern, K (2008)
Metal-organic coordination interactions in Fe-Terephthalic acid networks on Cu(100)
in Journal of the American Chemical Society (Print); ACS, American chemical society, Washington, DC (Stati Uniti d'America)
(literal)

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Tait, SL; Wang, Y; Costantini, G; Lin, N; Baraldi, A; Esch, F; Petaccia, L; Lizzit, S; Kern, K (literal)

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http://pubs.acs.org/doi/abs/10.1021/ja0778186?prevSearch=%255BContrib%253A%2Bbaraldi%255D&searchHistoryKey= (literal)

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\"[Tait, Steven L.; Wang, Yeliang; Costantini, Giovanni; Lin, Nian; Kern, Klaus] Max Planck Inst, Solid State Res, D-70569 Stuttgart, Germany; [Baraldi, Alessandro] Univ Trieste, Dept Phys, I-34127 Trieste, Italy; [Baraldi, Alessandro] Univ Trieste, Ctr Excellence Nanostructured Mat, I-34127 Trieste, Italy; [Baraldi, Alessandro; Esch, Friedrich] Lab TASC INFM CNR, Area Sci Pk, I-34012 Trieste, Italy; [Petaccia, Luca; Lizzit, Silvano] Sincrotrone Trieste SCpA, I-34012 Trieste, Italy; [Kern, Klaus] Ecole Polytech Fed Lausanne, Inst Phys & Nanostruct, CH-1015 Lausanne, Switzerland; [Costantini, Giovanni] Univ Warwick, Dept Chem, Coventry CV4 7AL, W Midlands, England (literal)

Titolo

Metal-organic coordination interactions in Fe-Terephthalic acid networks on Cu(100) (literal)

Abstract

Metal-organic coordination interactions are prime candidates for the formation of self-assembled, nanometer-scale periodic networks with room-temperature structural stability. We present X-ray photoelectron spectroscopy measurements of such networks at the Cu(1 00) surface which provide clear evidence for genuine metal-organic coordination. This is evident as binding energy shifts in the O 1s and Fe 3p photoelectron peaks, corresponding to O and Fe atoms involved in the coordination. Our results provide the first clear evidence for charge-transfer coordination in metal-organic networks at surfaces and demonstrate a well-defined oxidation state for the coordinated Fe ions. (literal)

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