On the Coupling of Vibrational Relaxation with the Dissociation-Recombination Kinetics: From Dynamics to Aerospace Applications. (Articolo in rivista)

Type
Label
  • On the Coupling of Vibrational Relaxation with the Dissociation-Recombination Kinetics: From Dynamics to Aerospace Applications. (Articolo in rivista) (literal)
Anno
  • 2004-01-01T00:00:00+01:00 (literal)
Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#doi
  • 10.1021/jp048847v (literal)
Alternative label
  • M. Capitelli ,G. Colonna ,F. Esposito (2004)
    On the Coupling of Vibrational Relaxation with the Dissociation-Recombination Kinetics: From Dynamics to Aerospace Applications.
    in The journal of physical chemistry. A; ACS, American chemical society, Washington, DC (Stati Uniti d'America)
    (literal)
Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#autori
  • M. Capitelli ,G. Colonna ,F. Esposito (literal)
Pagina inizio
  • 8930 (literal)
Pagina fine
  • 8934 (literal)
Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#url
  • http://cdn-pubs.acs.org/doi/abs/10.1021/jp048847v (literal)
Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#numeroVolume
  • 108 (literal)
Rivista
Note
  • Scopu (literal)
  • ISI Web of Science (WOS) (literal)
Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#affiliazioni
  • IMIP - Sezione di Bari (literal)
Titolo
  • On the Coupling of Vibrational Relaxation with the Dissociation-Recombination Kinetics: From Dynamics to Aerospace Applications. (literal)
Abstract
  • A refined set of state-to-state dissociation cross sections for the process N + N-2(v,j) --> 3N has been obtained by the quasiclassical trajectory (QCT) method and used in a 1D code describing the expansion of a dissociation-recombination mixture through a converging-diverging nozzle. The relevant vibrational kinetics includes V-V and V-T energy transfers as well as dissociation-recombination processes. The results show strong nonequilibrium vibrational distributions and non-Arrhenius dissociation rates along the nozzle axis as a consequence of the recombination process. (literal)
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