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On the Coupling of Vibrational Relaxation with the Dissociation-Recombination Kinetics: From Dynamics to Aerospace Applications. (Articolo in rivista)
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- On the Coupling of Vibrational Relaxation with the Dissociation-Recombination Kinetics: From Dynamics to Aerospace Applications. (Articolo in rivista) (literal)
- Anno
- 2004-01-01T00:00:00+01:00 (literal)
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#doi
- 10.1021/jp048847v (literal)
- Alternative label
M. Capitelli ,G. Colonna ,F. Esposito (2004)
On the Coupling of Vibrational Relaxation with the Dissociation-Recombination Kinetics: From Dynamics to Aerospace Applications.
in The journal of physical chemistry. A; ACS, American chemical society, Washington, DC (Stati Uniti d'America)
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- M. Capitelli ,G. Colonna ,F. Esposito (literal)
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- http://cdn-pubs.acs.org/doi/abs/10.1021/jp048847v (literal)
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- Titolo
- On the Coupling of Vibrational Relaxation with the Dissociation-Recombination Kinetics: From Dynamics to Aerospace Applications. (literal)
- Abstract
- A refined set of state-to-state dissociation cross sections for the process N + N-2(v,j) --> 3N has been obtained by the quasiclassical trajectory (QCT) method and used in a 1D code describing the expansion of a dissociation-recombination mixture through a converging-diverging nozzle. The relevant vibrational kinetics includes V-V and V-T energy transfers as well as dissociation-recombination processes. The results show strong nonequilibrium vibrational distributions and non-Arrhenius dissociation rates along the nozzle axis as a consequence of the recombination process. (literal)
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