Vapor phase processing of alpha-Fe2O3 photoelectrodes for water splitting: an insight into the structure/property interplay (Articolo in rivista)

Type

• Prodotto della ricerca (Classe)
• Articolo in rivista (Classe)

Label

• Vapor phase processing of alpha-Fe2O3 photoelectrodes for water splitting: an insight into the structure/property interplay (Articolo in rivista) (literal)

Anno

• 2015-01-01T00:00:00+01:00 (literal)

Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#doi

• 10.1021/acsami.5b00919 (literal)

Alternative label

• Warwick M.E.A; KaunistoK. K.; Barreca D.; Carraro G.; Gasparotto A.; Maccato C.; Bontempi E.; Sada C.; Ruoko T.-P.; Turner S.; Van Tendeloo G. (2015)
  Vapor phase processing of alpha-Fe2O3 photoelectrodes for water splitting: an insight into the structure/property interplay
  in ACS applied materials & interfaces (Online)
  (literal)

Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#autori

• Warwick M.E.A; KaunistoK. K.; Barreca D.; Carraro G.; Gasparotto A.; Maccato C.; Bontempi E.; Sada C.; Ruoko T.-P.; Turner S.; Van Tendeloo G. (literal)

Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#altreInformazioni

• Autori stranieri (literal)

Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#url

• http://pubs.acs.org/doi/abs/10.1021/acsami.5b00919 (literal)

Rivista

• ACS applied materials & interfaces (Rivista)

Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#affiliazioni

• 1,2,4-6 : Department of Chemistry, Padova University and INSTM, 35131 Padova, Italy / 2,9 : Department of Chemistry and Bioengineering, Tampere University of Technology, 33101 Tampere, Finland / 3 : CNR-IENI, Department of Chemistry, Padova University and INSTM, 35131 Padova, Italy / 7 : Chemistry for Technologies Laboratory, University of Brescia, 25123 Brescia, Italy / 8 : Department of Physics and Astronomy, Padova University, 35131 Padova, Italy / 10,11 : EMAT, University of Antwerp, 2020 Antwerpen, Belgium (literal)

Titolo

• Vapor phase processing of alpha-Fe2O3 photoelectrodes for water splitting: an insight into the structure/property interplay (literal)

Abstract

• Harvesting radiant energy to trigger water photoelectrolysis and produce clean hydrogen is receiving increasing attention in the search of alternative energy resources. In this regard, hematite (?-Fe2O3) nanostructures with controlled nano-organization have been fabricated and investigated for use as anodes in photoelectrochemical (PEC) cells. The target systems have been grown on conductive substrates by plasma enhanced-chemical vapor deposition (PE-CVD) and subjected to eventual ex-situ annealing in air to further tailor their structure and properties. A detailed multi-technique approach has enabled to elucidate the interrelations between system characteristics and the generated photocurrent. The present ?-Fe2O3 systems are characterized by a high purity and hierarchical morphologies consisting of nanopyramids/organized dendrites, offering a high contact area with the electrolyte. PEC data reveal a dramatic response enhancement upon thermal treatment, related to a more efficient electron transfer. The reasons underlying such a phenomenon are elucidated and discussed by transient absorption spectroscopy (TAS) studies of photogenerated charge carrier kinetics, investigated on different time scales for the first time on PE-CVD Fe2O3 nanostructures. (literal)

Prodotto di

• Modeling computazionale di sistemi complessi costituiti da molecole interagenti con superfici e nanosistemi (PM.P05.007.002) (Modulo)
• Institute of Condensed Matter Chemistry and Energy Technologies (ICMATE) (Istituto)

Autore CNR

• DAVIDE BARRECA (Persona)

Insieme di parole chiave

• Parole chiave di "Vapor phase processing of alpha-Fe2O3 photoelectrodes for water splitting: an insight into the structure/property interplay" (Insieme di parole chiave)

Incoming links:

Autore CNR di

• DAVIDE BARRECA (Persona)

Prodotto

• Institute of Condensed Matter Chemistry and Energy Technologies (ICMATE) (Istituto)
• Modeling computazionale di sistemi complessi costituiti da molecole interagenti con superfici e nanosistemi (PM.P05.007.002) (Modulo)

Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#rivistaDi

• ACS applied materials & interfaces (Rivista)

Insieme di parole chiave di

• Parole chiave di "Vapor phase processing of alpha-Fe2O3 photoelectrodes for water splitting: an insight into the structure/property interplay" (Insieme di parole chiave)