High-order harmonic spectroscopy for molecular imaging of polyatomic molecules (Articolo in rivista)

Type
Label
  • High-order harmonic spectroscopy for molecular imaging of polyatomic molecules (Articolo in rivista) (literal)
Anno
  • 2014-01-01T00:00:00+01:00 (literal)
Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#doi
  • 10.1039/c4fd00033a (literal)
Alternative label
  • Negro, M.; Devetta, M.; Facciala, D.; De Silvestri, S.; Vozzi, C.; Stagira, S. (2014)
    High-order harmonic spectroscopy for molecular imaging of polyatomic molecules
    in Faraday discussions (Print)
    (literal)
Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#autori
  • Negro, M.; Devetta, M.; Facciala, D.; De Silvestri, S.; Vozzi, C.; Stagira, S. (literal)
Pagina inizio
  • 133 (literal)
Pagina fine
  • 143 (literal)
Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#url
  • http://www.scopus.com/record/display.url?eid=2-s2.0-84912003501&origin=inward (literal)
Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#numeroVolume
  • 171 (literal)
Rivista
Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#pagineTotali
  • 11 (literal)
Note
  • ISI Web of Science (WOS) (literal)
  • Scopu (literal)
Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#affiliazioni
  • Consiglio Nazionale delle Ricerche (CNR); Polytechnic University of Milan (literal)
Titolo
  • High-order harmonic spectroscopy for molecular imaging of polyatomic molecules (literal)
Abstract
  • High-order harmonic generation is a powerful and sensitive tool for probing atomic and molecular structures, combining in the same measurement an unprecedented attosecond temporal resolution with a high spatial resolution of the order of an angstrom. Imaging of the outermost molecular orbital by high-order harmonic generation has been limited for a long time to very simple molecules, like nitrogen. Recently we demonstrated a technique that overcame several of the issues that have prevented the extension of molecular orbital tomography to more complex species, showing that molecular imaging can be applied to a triatomic molecule like carbon dioxide. Here we report on the application of such a technique to nitrous oxide (N2O) and acetylene (C2H2). This result represents a first step towards the imaging of fragile compounds, a category which includes most of the fundamental biological molecules. (literal)
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