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CVD precursors for transition metal oxide nanostructures: Molecular properties, surface behavior and temperature effects (Articolo in rivista)
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- CVD precursors for transition metal oxide nanostructures: Molecular properties, surface behavior and temperature effects (Articolo in rivista) (literal)
- Anno
- 2014-01-01T00:00:00+01:00 (literal)
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#doi
- 10.1002/pssa.201330085 (literal)
- Alternative label
Tabacchi G.; Fois E.; Barreca D.; Gasparotto A. (2014)
CVD precursors for transition metal oxide nanostructures: Molecular properties, surface behavior and temperature effects
in Physica status solidi. A, Applications and materials science (Print)
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- Tabacchi G.; Fois E.; Barreca D.; Gasparotto A. (literal)
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- Invited Paper; Selezionato per la Cover Image (Physica Status Solidi A, 2014, 211, 241-524).
in SCOPUS indicizzato come (Conference Paper) (literal)
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- http://onlinelibrary.wiley.com/doi/10.1002/pssa.201330085/abstract;jsessionid=329F5C1426A88A5684F4941B42AB8307.f03t01 (literal)
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- 1,2 : Department of Science and High Technology, Insubria University and INSTM, 22100 Como, Italy /
3 : CNR-IENI and INSTM, Department of Chemistry, Padova University, 35131 Padova, Italy /
4 : Department of Chemistry, Padova University, INSTM, 35131 Padova, Italy (literal)
- Titolo
- CVD precursors for transition metal oxide nanostructures: Molecular properties, surface behavior and temperature effects (literal)
- Abstract
- Integrated analyses on a series of ?-diketonate-diamine transition metal complexes (M = Fe, Co, Cu, Zn) highlight the metal center influence on molecular physico-chemical properties and provide understanding of the favorable behavior of these compounds as precursors in the chemical vapor deposition (CVD) growth of metal/metal oxide nanomaterials. The Zn complex, which shows the most symmetric coordination environment in the gas phase, is activated in contact with the heated CVD growth surface model. First-principles simulations evidenced surface-induced rolling motion of the Zn precursor in the 363-750 K range, suggesting the relevance of vibrationally excited molecular rolling as activation pathway in high temperature surface chemistry. Molecular properties (left) and hot-surface behavior (right) of the Zn(hfa)2TMEDA CVD precursor. (literal)
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