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Nitrocatechol/ZnO interface: The role of dipole in a dye/metal-oxide model system (Articolo in rivista)
- Type
- Label
- Nitrocatechol/ZnO interface: The role of dipole in a dye/metal-oxide model system (Articolo in rivista) (literal)
- Anno
- 2014-01-01T00:00:00+01:00 (literal)
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#doi
- 10.1021/jp410376r (literal)
- Alternative label
Arnaud G. F. [ 1,2 ] ; De Renzi V. [ 1,2 ] ; del Pennino U. [ 1,2 ] ; Biagi R. [ 1,2 ] ; Corradini V. [ 2 ] ; Calzolari A. [ 2,3 ] ; Ruini A. [ 2,1 ] ; Catellani A. [ 2,4 ] (2014)
Nitrocatechol/ZnO interface: The role of dipole in a dye/metal-oxide model system
in Journal of physical chemistry. C
(literal)
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#autori
- Arnaud G. F. [ 1,2 ] ; De Renzi V. [ 1,2 ] ; del Pennino U. [ 1,2 ] ; Biagi R. [ 1,2 ] ; Corradini V. [ 2 ] ; Calzolari A. [ 2,3 ] ; Ruini A. [ 2,1 ] ; Catellani A. [ 2,4 ] (literal)
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- Note
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- [ 1 ] Univ Modena & Reggio Emilia, Dipartimento Sci Fis Informat & Matemat, I-41125 Modena, Italy
[ 2 ] CNR NANO, Ist Nanosci, I-41125 Modena, Italy
[ 3 ] Univ N Texas, Dept Phys, Denton, TX 76203 USA
[ 4 ] CNR IMEM, I-43100 Parma, Italy (literal)
- Titolo
- Nitrocatechol/ZnO interface: The role of dipole in a dye/metal-oxide model system (literal)
- Abstract
- The electronic properties of a prototype system suitable for dye-sensitized solar cell applications are investigated both experimentally and theoretically by means of electron spectroscopies (high-resolution electron energy loss spectroscopy, HREELS, and ultraviolet and X-ray photoemission spectroscopies, UPS and XPS) and first-principles density functional theory (DFT)-based calculations. The comparison of HREELS and UPS data with the DFT results allows the microscopic description of electronic structure modifications upon interface formation, and provides a quantitative evaluation of the ionization energy and electron affinity changes induced by functionalization: these variations can be associated to the electric dipole of the functional species and, thus, to the formation of an interface dipole layer. © 2014 American Chemical Society. (literal)
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