http://www.cnr.it/ontology/cnr/individuo/prodotto/ID265721
The trigonal form of i-PP in random C3/C5/C6 terpolymers (Articolo in rivista)
- Type
- Label
- The trigonal form of i-PP in random C3/C5/C6 terpolymers (Articolo in rivista) (literal)
- Anno
- 2013-01-01T00:00:00+01:00 (literal)
- Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#doi
- 10.1016/j.polymer.2013.01041 (literal)
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- Boragno L.;Stagnaro P.;Forlini F;Azzurri F; Alfonso G.C (literal)
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- ISI Web of Science (WOS) (literal)
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- Boragno L Stagnaro P ISMAC Genova
Forlini F ISMAC Milano
Azzurri F. Alfonso G.C. Università di Genova (literal)
- Titolo
- The trigonal form of i-PP in random C3/C5/C6 terpolymers (literal)
- Abstract
- The formation of the trigonal structure of isotactic polypropylene (i-PP) in a series of random terpolymers
of propylene (C3) with n-pentene-1 (C5) and n-hexene-1 (C6) by cooling from the molten state was
investigated with the aim of assessing to what extent the intrinsic molecular disorder and the length of
the side branch of the comonomers reflect on structuring kinetics and features of the crystal lattice.
Experiments were performed on samples with an overall content of comonomers of ca. 25 mol% and
show that, alike in the random copolymers of propylene with 1-pentene (C3/C5) or with 1-hexene (C3/
C6), the trigonal modification of i-PP, delta form, develops upon cooling from the molten state also in the
case of random terpolymers. At a constant molar fraction of propylene, the values of a and b axes of the
unit cell linearly depend on the relative proportion of the two comonomers. Crystallinity and cell constant
values as a function of terpolymer composition were provided by evaluation of data obtained from
deconvoluted WAXD patterns. The development of crystallinity in isothermal conditions was followed at
0 and 20 ?°C, both by WAXD and DSC. Results were compared with those of the correspondent C3/C5 and
C3/C6 copolymers and used to confirm the kinetic model proposed in a previous paper. (literal)
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