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The oxygen isotope exchange between carbon dioxide and water in the Larderello geothermal field (Italy) during fluid reinjection. (Articolo in rivista)
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- The oxygen isotope exchange between carbon dioxide and water in the Larderello geothermal field (Italy) during fluid reinjection. (Articolo in rivista) (literal)
- Anno
- 2011-01-01T00:00:00+01:00 (literal)
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- Titolo
- The oxygen isotope exchange between carbon dioxide and water in the Larderello geothermal field (Italy) during fluid reinjection. (literal)
- Abstract
- The oxygen isotope compositions of CO2 and water vapor samples collected from Larderello geothermal
wells after the start of the fluid reinjection program suggest that if the oxygen isotope exchange in the
vapor phase does, in fact, exist, it is a very slow process when compared with the residence time of
the fluids in the geothermal reservoir. This is because carbon dioxide and water vapor phases could
not have equilibrated significantly in the vapor-dominated reservoir. This conclusion implies that the
oxygen isotope composition of carbon dioxide may possibly be used as a tool in geothermal exploration
for revealing the presence of liquid water in deep geothermal systems. Based on the interpretation of the
oxygen isotope data of the CO2, I propose that the origin of the low oxygen isotope ratios of carbon dioxide
at Larderello is the high-temperature exchange with liquid water in the lower reservoir. In Larderello, the
liquid water-rock interaction in the lower reservoir may have increased the 18O/16O ratio of the recharge
meteoric component. By contrast, lack of high-temperature liquid water in the upper reservoir suggests
that the large \"?18Oshift\" described for the upper-reservoir steam during the last decades reflects varying
degrees of dilution of the lower-reservoir fluid by the low-18O vaporized liquid water of meteoric origin
that recharges the field at shallow depth, with local contribution from still deeper high-18O water vapor
of magmatic origin. The low oxygen isotope composition of the Mesozoic carbonaceous rocks that form
the upper reservoir, consequently, likely represents a \"fossil\" record of the past hot-water geothermal
stage.
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