Process Intensification by Membrane Reactors: High-Temperature Water Gas Shift Reaction as Single Stage for Syngas Upgrading (Articolo in rivista)

Type
Label
  • Process Intensification by Membrane Reactors: High-Temperature Water Gas Shift Reaction as Single Stage for Syngas Upgrading (Articolo in rivista) (literal)
Anno
  • 2012-01-01T00:00:00+01:00 (literal)
Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#doi
  • 10.1002/ceat.201100641 (literal)
Alternative label
  • Brunetti A.; Caravella A.; Drioli E.; Barbieri G. (2012)
    Process Intensification by Membrane Reactors: High-Temperature Water Gas Shift Reaction as Single Stage for Syngas Upgrading
    in Chemical engineering & technology
    (literal)
Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#autori
  • Brunetti A.; Caravella A.; Drioli E.; Barbieri G. (literal)
Pagina inizio
  • 1238 (literal)
Pagina fine
  • 1248 (literal)
Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#numeroVolume
  • 35 (literal)
Rivista
Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#pagineTotali
  • 11 (literal)
Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#numeroFascicolo
  • 7 (literal)
Note
  • ISI Web of Science (WOS) (literal)
  • Scopu (literal)
Http://www.cnr.it/ontology/cnr/pubblicazioni.owl#affiliazioni
  • National Research Council, Institute for Membrane Technology (ITM-CNR), Rende, Italy University of Calabria, Department of Chemical Engineering and Materials, Rende, Italy National Institute of Advanced Industrial Science and Technology (AIST), Research Institute for Innovation in Sustainable Chemistry, Tsukuba (Ibaraki), Japan (literal)
Titolo
  • Process Intensification by Membrane Reactors: High-Temperature Water Gas Shift Reaction as Single Stage for Syngas Upgrading (literal)
Abstract
  • Pd-based membrane reactors (MRs) selectively removing hydrogen shift the equilibrium conversion of this new reactor type to values higher than those imposed by thermodynamics to traditional reactors. Thus, the equilibrium conversion of CO is significantly increased and can be very strongly depending on the hydrogen extracted also at a higher temperature. This property of the MRs offers important benefits also in terms of process intensification. In the typical high-temperature range for this reaction, i.e., 300-450°C, the performance of an MR turned out to be so effective that the two reactors of a traditional process can be replaced by one MR of lower volume, too. The conversion of the MR is higher than the one of the whole traditional process which includes a heat exchanger in addition to two reactors. Consequently, less and smaller unit operations are required when an MR operates the water gas shift reaction pursuing the process intensification philosophy. (literal)
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